I've got the latest Powered Up remote, I was hoping it would pair with the Move Hub instead of using the Boost App.
At the moment it doesn't want to pair.
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This is not possible at the moment. This could be enabled in a future firmware update, but I'm honestly not sure how this would work. The Move Hub has 4 possible outputs. Mapping those to the pair of outputs normally controlled by the current remote seems like it would be somewhat clunky or non-intuitive.
If you use third party software to form a Powered Up network you can pair the remote and the Move hub to a computer and control them both from there. You could write your program such that pressing the green button would change the LED colour and swap between controlling ports A/B or C/D.